2021
DOI: 10.1021/acs.macromol.0c02740 View full text |Buy / Rent full text
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Abstract: We provide a perspective on polymer glass formation, with an emphasis on models in which the fluid entropy and collective particle motion dominate the theoretical description and data analysis. The entropy theory of glass formation has its origins in experimental observations relating to correlations between the fluid entropy and liquid dynamics going back nearly a century ago, and it has entered a new phase in recent years. We first discuss the dynamics of liquids in the high-temperature Arrhenius regime, whe… Show more

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